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Didn't you ask this on the emergeny-board...?
Well, there are examples in some stories of Chaos followers devouring spirit stones so I think it's possible.
Well at the end of Medusa V Elarique's soul got captured by chaos so now she gets tormented for all eternity.
I think its possible to break it yes. My friends and i have fun doing "corpse hits" when one of my squads get overkilled and I always write in something about spirit stones getting smashed when that happens.
Check out my Codex: Farmyard Animals here!
If anyone wants any kind of help writing fluff for any kind of GW army just ask.