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I'm sorry but I can't get that image to load. You should try to use photobucket as they tend to be easy to upload for others to see. Then we can tell you what we think.
I actually really like that scheme. Inverted trim/flat surfaces - looks really good.
for example, on some of the marines, the shin guard should be purple, rather than the knee pad. On some of them, the shoulders/trims should be inverted and on some of them, the heads should be purple.
The variety will give you a better impression that they are chaos space marines rather than the more strictly organized loyal ones. I mean, Noise Marines are farther away from 'Codex Chapter' than the space wolves.
That looks good. I the black and purple will work well as Slaanesh. I agree that they could be made to be a little less uniform here and there. But only do that if you feel good about it. If you like the idea of uniform then keep them that way. I do see no eye colour. You could try to give them glowing green eyes or blue eyes. It might make them look more unusual and therefore more chaotic.
I actually had them with green eyes in the first pic that didnt work.
I forgot to put them in the second pic.
Chaos - 11W 0L 0D
Orks - 8W 0L 0D
Tyranids - 8W 0L 0D